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dc.contributor.authorSilva, Franciscarlos Gomes da-
dc.contributor.authorVasilakaki, Marianna-
dc.contributor.authorGomes, Rafael Cabreira-
dc.contributor.authorAquino, Renata-
dc.contributor.authorCampos, Alex Fabiano Cortez-
dc.contributor.authorDubois, Emmanuelle-
dc.contributor.authorPerzynski, Régine-
dc.contributor.authorDepeyrot, Jérôme-
dc.contributor.authorTrohidou, Kalliopi-
dc.date.accessioned2022-09-19T20:24:05Z-
dc.date.available2022-09-19T20:24:05Z-
dc.date.issued2022-08-04-
dc.identifier.citationSILVA, Franciscarlos Gomes da et al. A numerical study on the interplay between the intra-particle and interparticle characteristics in bimagnetic soft/soft and hard/soft ultrasmall nanoparticle assemblies. Nanoscale Advances, v. 4, n. 18, p. 3777-3785, 2022. DOI 10.1039/D1NA00894C. Disponível em: https://pubs.rsc.org/en/content/articlelanding/2022/NA/D1NA00894C. Acesso em: 19 set. 2022.pt_BR
dc.identifier.urihttps://repositorio.unb.br/handle/10482/44851-
dc.language.isoInglêspt_BR
dc.publisherRoyal Society of Chemistrypt_BR
dc.rightsAcesso Abertopt_BR
dc.titleA numerical study on the interplay between the intra-particle and interparticle characteristics in bimagnetic soft/soft and hard/soft ultrasmall nanoparticle assembliespt_BR
dc.typeArtigopt_BR
dc.subject.keywordBimagnéticopt_BR
dc.subject.keywordNanoestruturaspt_BR
dc.subject.keywordNanopartículas - propriedades magnéticaspt_BR
dc.rights.licenseNanoscale Advances - This article is licensed under a Creative Commons Attribution-NonCommercial 3.0 Unported Licence. FONTE: https://pubs.rsc.org/en/content/articlelanding/2022/NA/D1NA00894C. Acesso em: 19 set. 2022.pt_BR
dc.identifier.doihttps://doi.org/10.1039/D1NA00894Cpt_BR
dc.description.abstract1Amesoscopic scale approach and the Monte Carlo (MC)method have been employed to study the exchange bias behaviour of MnFe2O4 (soft)/maghemite (soft) and CoFe2O4 (hard)/maghemite (soft) nanoparticles (NPs) of size ~ 3nm in dense and diluted assemblies at low temperatures. The analysis of our MC results clearly shows that in the powder samples the contribution to the exchange bias field (Hex) and the coercivity (Hc) comes mainly from the intraparticle core/shell structure in the hard/soft sample and that the interplay between the internal characteristics and the interparticle interactions is more important in the soft/soft samples where the dipolar strength is enhanced. In the diluted frozen ferrofluid samples where interparticle exchange interactions are absent and the role of the dipolar interactions is not significant the exchange bias effects are reduced, and they come from the intra particle structure. The variation of Hex and Hc with the applied cooling field well reproduces the experimental findings and sheds light on the key mechanisms of the observed magnetic behaviour. Our results demonstrate the possibility to control the magnetic behaviour of nanostructures by using properly chosen core/shell bimagnetic nanoparticles.pt_BR
dc.identifier.orcidhttps://orcid.org/0000-0003-1976-867Xpt_BR
dc.identifier.orcidhttps://orcid.org/0000-0003-1832-7549pt_BR
dc.identifier.orcidhttps://orcid.org/0000-0002-7918-8522pt_BR
dc.identifier.orcidhttps://orcid.org/0000-0001-8554-8486pt_BR
dc.identifier.orcidhttps://orcid.org/0000-0002-6634-6245pt_BR
dc.identifier.orcidhttps://orcid.org/0000-0002-1689-573Xpt_BR
dc.identifier.orcidhttps://orcid.org/0000-0002-6921-5419pt_BR
dc.contributor.emailmailto:franciscarlos@fis.unb.brpt_BR
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